The nonlinear large-eddy simulation (nLES) method is extended here to simulations of
Sc ≈ 1 and
Sc⪢1 turbulent mixing of passive-scalar fields. These are the first LES studies to reproduce the instantaneous structure of the scalar-energy field
?start
2end?(x,t) at viscous-convective scales in the high Schmidt-number regime. The simulations employ a refinement of the nLES method with multifractal modeling first proposed by
G. C. Burton and W. J. A. Dahm [Phys. Fluids 17, 075111 (2005)]
. In this approach, the nonlinear inertial stresses

in the filtered Navier–Stokes equation and the nonlinear scalar fluxes

in the filtered advection-diffusion equation are calculated directly, using multifractal models for the subgrid velocity and scalar fields,
ujsgs and
ϕsgs. Resolved energy levels are controlled by a new adaptive backscatter limiter that adjusts locally to changing flow conditions consistent with the mechanism governing energy transfer in actual hydrodynamic turbulence. No artificial viscosity or diffusivity closures are applied and no explicit de-aliasing is performed. The nLES approach is shown to simulate accurately
Sc ≈ 1 mixing for flows between
Reλ ≈ 35 and 4100, the highest
Reλ tested. Characteristics of the resulting scalar field are examined, including the turbulence-to-scalar time-scale ratio and total scalar variance
〈ϕ′2〉, indicating good agreement with prior studies. Simulations between
Sc = 8 and 8192 produce the first scalar-energy spectra from an LES that exhibit
k−1 scaling in the viscous-convective range, consistent with the analytical prediction of
G. K. Batchelor [J. Fluid Mech. 5, 113 (1959)]
. The simulations indicate decreasing scalar anisotropy and increasing intermittency with increasing Schmidt number, also consistent with prior studies.